Publication:
Source Data for Self-Spinning Filaments for Autonomously Linked Microfibers

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dc.contributor.authorBarber, Dylan M
dc.contributor.authorEmrick, Todd S.
dc.contributor.authorGrason, Gregory
dc.contributor.authorCrosby, Alfred
dc.contributor.departmentUniversity of Massachusetts Amherst
dc.contributor.departmentUniversity of Massachusetts Amherst
dc.contributor.departmentUniversity of Massachusetts Amherst
dc.contributor.departmentUniversity of Massachusetts Amherst
dc.date2024-01-04T19:19:17.000
dc.date.accessioned2024-04-26T11:06:41Z
dc.date.available2024-04-26T11:06:41Z
dc.date.issued2022-01-01
dc.description<p>README.txt included in .zip file. This paper is currently available in ChemRxiv.</p>
dc.description.abstractFilamentous bundles are ubiquitous in Nature, achieving highly adaptive functions and structural integrity from assembly of diverse mesoscale supramolecular elements. Engineering routes to synthetic, topologically integrated analogs demands precisely coordinated control of multiple filaments’ shapes and positions, a major challenge when performed without complex machinery or labor-intensive processing. Here, we demonstrate a photocreasing design that encodes local curvature and twist into mesoscale polymer filaments, enabling their programmed transformation into target 3-dimensional geometries. Importantly, patterned photocreasing of filament arrays drives autonomous spinning to form linked filament bundles that are highly entangled and structurally robust. In individual filaments, photocreases unlock paths 16 to arbitrary, 3-dimensional curves in space. Collectively, photocrease-mediated bundling establishes a transformative paradigm enabling smart, self-assembled mesostructures that mimic performance-differentiating structures in Nature (e.g., tendon and muscle fiber) and the macro-engineered world (e.g., rope).
dc.description.sponsorship1) NDSEG Fellowship 2) NSF DMR 2028885 3) W911NF-15-1-0358
dc.identifier.doihttps://doi.org/10.7275/6ybn-g003
dc.identifier.orcidBarber: 0000-0001-6129-5779
dc.identifier.urihttps://hdl.handle.net/20.500.14394/10664
dc.relationhttps://doi.org/10.26434/chemrxiv-2022-dhd35
dc.source.statuspublished
dc.subjectself-assembly
dc.subjectmesoscale
dc.subjectelastocapillarity
dc.subjectstimulus response
dc.subjectbundling
dc.subjectApplied Mechanics
dc.subjectMaterials Chemistry
dc.subjectPolymer and Organic Materials
dc.subjectPolymer Chemistry
dc.titleSource Data for Self-Spinning Filaments for Autonomously Linked Microfibers
dc.typedata
dc.typearticle
digcom.contributor.authorisAuthorOfPublication|email:dylan.m.barber4@gmail.com|institution:University of Massachusetts Amherst|Barber, Dylan M
digcom.contributor.authorisAuthorOfPublication|email:tsemrick@mail.pse.umass.edu|institution:University of Massachusetts Amherst|Emrick, Todd S.
digcom.contributor.authorisAuthorOfPublication|email:grason@mail.pse.umass.edu|institution:University of Massachusetts Amherst|Grason, Gregory
digcom.contributor.authorisAuthorOfPublication|email:crosby@mail.pse.umass.edu|institution:University of Massachusetts Amherst|Crosby, Alfred
digcom.identifierdata/159
digcom.identifier.contextkey32464406
digcom.identifier.submissionpathdata/159
dspace.entity.typePublication
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relation.isAuthorOfPublication5226f9e1-9975-482b-ad43-e544f48c6eef
relation.isAuthorOfPublication.latestForDiscoverybac50549-1dcf-4279-81ae-d0063fe29173
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